SSGF Magazine 2013

STEWARDSHIP
SCIENCE
The SSGF Magazine
PRESSURE
PREDICTIONS
How Sandia is refining matter models
by applying first principles
Los Alamos: Neutron
beam record-breaker
Livermore: At the edge
of the periodic table
Plus: Former fellow goes to Washington,
more juice for Z, bringing the big bang
down to size, fission and scission, and
SSGF on the road.
2013-2014
Department of Energy National Nuclear Security Administration
Stewardship Science
Graduate Fellowship
The Department of Energy National Nuclear Security Administration Stewardship Science
Graduate Fellowship (DOE NNSA SSGF) program provides outstanding benefits and
opportunities to students pursuing a Ph.D. in areas of interest to stewardship science,
such as properties of materials under extreme conditions and hydrodynamics, nuclear science,
or high energy density physics. The fellowship includes a 12-week research experience
at Lawrence Livermore National Laboratory,
Los Alamos National Laboratory
or Sandia National Laboratories.
APPLICATIONS DUE
MID JANUARY
BENEFITS
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Payment of full tuition and required fees
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Renewable up to four years
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IMAGES
LEFT: A metallic case
called a hohlraum holds the fuel
capsule for National Ignition Facility
experiments at Lawrence
Livermore National Laboratory.
MIDDLE: At Sandia National
Laboratories, high magnetic
fields on the aluminum side of this
magnetically launched aluminum/copper
flyer drive it into diamond targets at
tens of kilometers per second,
generating enormous pressures and
shock waves in the diamond.
RIGHT: X-ray laser flashes generated in
an undulator, an arrangement of magnets
that directs high-energy electrons. Image
courtesy of Los Alamos
National Laboratory.
The DOE NNSA SSGF program is open to senior undergraduates or students in their first or second year of
graduate study. Access application materials and additional information at:
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This is an equal opportunity program and is open to all qualified persons without regard to race, gender, religion, age, physical disability or national origin.
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National Nuclear Security Administration
LETTER FROM NNSA
Investing in the Future

MUCH OF the discussion in Washington these days revolves around
fiscal restraint, doing more with less and the dreaded S word: sequestration.
Even in this environment, there is a continuing understanding of the value
of science by NNSA leadership and the nations elected representatives.
This fourth edition of Stewardship Science: The SSGF Magazine represents a
milestone since the magazines publication now spans an entire class of
fellows! Our shared commitment to sustaining programs like the Stewardship
Science Graduate Fellowship represents the value we place on developing the
leaders of tomorrows scientific endeavors. The work highlighted in this issue
shows the return on those investments.
Christopher Deeney
In missions that range from reducing the risks of nuclear terrorism or the
proliferation of nuclear weapons technology to responding to nuclear accidents like the
one at Fukushima in Japan, NNSA relies on tools and technology based on a fundamental
understanding of nuclear science. The work of fellow Matthew Buckner at Lawrence
Livermore National Laboratory (page 4) on Accelerator Mass Spectrometry (AMS) advances
the state-of-the-art of a key diagnostic tool. AMS is used in several fields, including
detecting signatures of nuclear fuel reprocessing an important nonproliferation
function. Matthew used AutoCAD, along with simulation tools, to build a prototype
detector, install it and test it on a Livermore accelerator beamline.
At a more fundamental level, fellow Nicole Fields worked on calibrating a key material
during her research practicum at Los Alamos National Laboratory (page 7). Fields
examined germanium-76, an isotope researchers hope will find evidence of neutrinoless
double-beta decay. This rare interaction is key to understanding neutrinos and can
help in advancing our fundamental knowledge of the universe. She used neutron beams
from LANSCE, the Los Alamos Neutron Science Center, to simulate cosmic ray exposure
so she could calibrate the effects of this radiation for future experiments.
In related work, fellow Joshua Renner conducted his practicum at Livermore (page 7) on
the technology for time projection chambers (TPCs). These TPCs also are designed
to detect evidence of neutrinoless double-beta decay. Renner worked with physicist Adam
Bernstein on the negative ion TPC and used simulation tools to emulate ion drift behavior.
These tools provided clues to help maximize the efficiency of Livermores detector for
these rare interactions.
From fundamental exploration to prototype development, Stewardship Science fellows
are advancing the frontiers of nuclear science and helping NNSA build its future.
Christopher Deeney
Assistant Deputy Administrator
for Stockpile Stewardship
U.S. Department of Energy National
Nuclear Security Administration
With assistance from Mark Visosky

Senior Technical Advisor
TechSource, Inc., contractor to NNSA
S TEWA R D S H I P S C I EN C E 13/ 14 TH E S SG F MA G A ZI NE PC
STEWARDSHIP
SCIENCE
The SSGF Magazine
2013 - 2014
FEATURES
LAB INITIO
10
By Jacob Berkowitz
Sandias Luke Shulenburger and colleagues are harnessing the power of quantum Monte
Carlo methods to boost matter models accuracy. Theyre already finding that elements
under extreme temperatures and pressures behave in unexpected ways.
IN THEIR ELEMENT
15
By Karyn Hede
The newest, heaviest elements on the periodic table are difficult to produce and often
quickly disappear, making it hard to quantify their properties. Livermore scientists are
finding new ways to separate and understand these strange substances.
THE BEAM COUNTERS
19
By Thomas R. ODonnell
Los Alamos National Laboratorys Trident, a powerful laser that produces fleeting pulses,
has racked up a new neutron beam record. The experiment could lead to more precise
detectors and to compact neutron sources for science and nuclear forensics.
COVER
Stewardship Science: The SSGF Magazine showcases researchers and graduate students at U.S.
Department of Energy National Nuclear Security Administration (DOE NNSA) national laboratories.
Stewardship Science is published annually by the Krell Institute for the NNSA Office of Defense
Sciences Stewardship Science Graduate Fellowship (SSGF) program, which Krell manages for NNSA
under cooperative agreement DE-FC52-08NA28752. Krell is a nonprofit organization serving the
STEWARDSHIP SCIENCE GRADUATE FELLOWSHIP
science, technology and education communities.
Copyright 2013 by the Krell Institute. All rights reserved.
For additional information, please visit www.krellinst.org/ssgf or contact the Krell Institute 1609
Golden Aspen Dr., Suite 101 | Ames, IA 50010 | Attn: SSGF | (515) 956-3696
STEWARDSHIP SCIENCE GRADUATE FELLOWSHIP
P 2 ST E WA RD SH IP SCIENCE 1 3 / 1 4 T HE S S GF M AGAZ INE
FIRST-PRINCIPLE INVESTIGATORS
This visualization by Sandia National Laboratories
Luke Shulenburger shows a charge density map
for FeO (iron oxide) calculated with quantum
Monte Carlo methods. Iron oxide is of interest
to geophysicists, but modeling its electronic
structure is challenging. Shulenburger belongs
to a corps of young mathematicians who
include Miguel Morales of Lawrence Livermore
National Laboratory, an alumnus of the National
Nuclear Security Administration Stewardship
Science Graduate Fellowship working out the
fundamental properties of this and other materials
based on first-principles physics. Read more
starting on page 10.
2013
2014
DEPARTMENTS
FRONT LINES
4 FISSION UP CLOSE

Deciphering the details of atom splitting.
FELLOWS ON LOCATION
The latest SSGF graduates design a detector, test elements for gamma
ray exposure, put tantalum under pressure, track some particles and
measure ion-stopping power.
24 BOTTLING THE SUN
5 Z, SUPERCHARGED

SAMPLINGS
Fellow Evan Davis probes the slim slice
Sandia plans to amp up the Z machine in the same space.
of turbulence that has an outsized say

in fusion energys viability.
6 LITTLE BIG BANG

Probing the properties of the quark-gluon plasma.
DIRECTORY
9 CONVERSATION: BRIDGING
SCIENCE, POLICY AND THE PUBLIC
25 DOE NNSA SSGF FELLOWS
Former fellow Laura Berzak Hopkins on providing science expertise to
Where to find current fellows
Congress, fusions two varieties and her Why-Sci communications project.
and alumni.
IMAGE CREDITS
Cover, Luke Shulenburger, Sandia
National Laboratories (SNL);
page 1, National Nuclear Security
Administration; page 4, Walid
Younes, Lawrence Livermore
National Laboratory (LLNL);
page 5, SNL; page 6, ATLAS
Experiment/CERN; page 9,
Laura Berzak Hopkins; pages
10-12, Shulenburger/SNL; pages
16-17, LLNL; pages 19-20,
Markus Roth, Technical
University of Darmstadt;
page 21, julsdesign (source:
[LANL]); pages 22-23, LANL.
EDITOR
Bill Cannon
SR. SCIENCE EDITOR
Thomas R. ODonnell
DESIGN
julsdesign, inc.
COPY READERS
Ron Winther
Shelly Olsan
CONTRIBUTING WRITERS
Monte Basgall
Jacob Berkowitz
Tony Fitzpatrick
Karyn Hede
Thomas R. ODonnell
Sarah Webb
SSGF STEERING COMMITTEE

Robert Voigt
Nuclear Security Division
SAIC
Darryl P. Butt
Department of Materials Science and Engineering
Boise State University
Stephen M. Sterbenz
Kimberly S. Budil
Lawrence Livermore National Laboratory
Ramon J. Leeper
Sandia National Laboratories
S TEWA R D S H I P S C I EN C E 13/ 14 TH E S S G F MA G A ZI NE P3
FRONT LINES
F E L L O W S O N L O C AT I O N
Fission Up Close
lthough it releases vast amounts of energy, the process
Members of DOE National Nuclear Security Administration

Stewardship Science Graduate Fellowships 2013 outgoing
class share their national lab research experience.
of splitting atomic nuclei is still difficult to understand

in detail. Nuclei are infinitesimally small and fission
happens incredibly quickly (within 10-20 seconds), so
its hard to study in a laboratory.
DETECTOR UPGRADE
Undaunted, Lawrence Livermore National Laboratory researchers are
Matthew Buckners practicum at Lawrence
looking at fissions microscopic detail with the hope of improving
Livermore National Laboratory was a bit like a
nuclear waste management and recycling and increasing nuclear power
high-tech physicists shop class. His plans for an
production. Describing fission in detail also can help answer basic
improved gas ionization chamber detector went
science questions, such as how heavy elements formed in the universe.
from computer modeling to fabrication

at a machine shop and testing.
Physicists started delving into fission theoretically 75 years ago by

simplifying the problem. Instead of looking at all the protons and
Buckner worked with Scott Tumey at Livermores Center for Accelerator
neutrons within the nucleus, they considered it as a liquid drop,
Mass Spectrometry. Accelerator mass spectrometry, or AMS, speeds ions
Livermores Walid
to high energies, separating isotopes from surrounding material before
Younes says. During
mass analysis. AMS is used in several fields, including detecting signatures
fission, the drop would
of nuclear fuel reprocessing an important nonproliferation function.
stretch into an oblong

peanut shape. At
The device Buckner made uses AMS to measure transition metal
the scission point,
activation products. He simulated a previous design on a computer
the narrow neck in
and found that voltages were incorrectly applied for the detector
the peanut would
anodes to adequately collect electrons. After some research, he used
break to form two
simulations to tailor the new detector design to transition metal
A schematic illustration of microscopic fission
new atomic nuclei
activation products and modified grids, voltages and other aspects.
calculations for plutonium-240. The arrows
and release energy.
represent evolution of the nucleus in the calculation

across its energy surface toward its breaking
point. On the right are three examples of the
nuclear configuration near breaking.
Using AutoCAD software, Buckner designed a detector enclosure
Even today, with
for fabrication at the labs machine shop, then built the detector and
high-performance
installed it on the accelerator beam line. He and Tumey tested it
computers, the
with relevant materials and Buckner compared its resolving power
data challenges for
with that of the original detector. The new detector is more sensitive
understanding fission remain enormous. If you put all that information
and bolsters the labs nuclear forensics capabilities, Tumey says.
into a computer, Younes says, youd quickly be looking at tens of millions

of processor hours as the simulation moves toward scission.
The fellow, meanwhile, says the project was a contrast with his doctoral
work at the University of North Carolina at Chapel Hill. Under
Despite the difficulty, Younes and his colleagues have extended the
Christian Iliadis, Buckner has studied proton capture by rare oxygen
traditional droplet model. Instead of considering the nucleus as a
isotopes thermonuclear reactions associated with nucleosynthesis
single stretching blob, their calculation includes protons and neutrons
and energy generation in a class of stars and with explosive hydrogen
that arrange themselves within the droplet in a way thats energetically
burning during classical novae. During the summer, he reports, it
favorable. They then stretch the theoretical nucleus until it breaks
was really interesting to participate in an application of the nuclear
naturally and probe how that force affects the individual particles.
and accelerator physics Im interested in.
We dont force it, he says. We dont take a knife and cut it in two.
continued on page 6
continued on page 7
Z, Supercharged
y far the worlds largest, most powerful and most
four stages of pulse compression must reduce the span of the Marx
successful pulsed-power accelerator, Sandia National
pulse. Pulse-compression hardware introduces electrical impedance
Laboratories Z machine is poised to become even
mismatches, causing multiple internal reflections of the Z power pulse
more powerful.
and reducing Zs efficiency. In addition, Stygar says, pulse compression

hardware substantially complicates the design of a machine like Z,
The Z machine named for z-pinch, a type of plasma device driven by
increasing maintenance costs and ramping up the difficulty of
pulsed-power accelerators generates an 80-terawatt electrical power
developing an accurate accelerator circuit model and conducting
pulse. Its 33 meters in diameter and fills the high bay of Building
accelerator simulations.
983 on the labs Albuquerque, N.M., campus. Thanks to LTD technology,

for linear transformer driver, over time Z will become Z 300, a
An LTD generates a 100-nanosecond power pulse in a single step,
300-terawatt machine that will fit the same space.
which eliminates the need for additional pulse-compression hardware,

Stygar says. As a result, an LTD module is twice as efficient as a
The Z 300 will generate twice the current and four times the power that
Marx-driven module, substantially more compact, less costly to
Z now generates, says William Stygar, manager of the labs Advanced
maintain and easier to simulate.
Accelerator Physics Department, which specializes in pulsed-power

accelerator physics. With that capability, Z 300 will be able to perform
The belly of the LTD beast is a collection of 20 bricks arrayed in a
ultra-precise high energy density physics experiments in support of
circle like the spokes of a wheel. Each shoebox-sized brick holds a
various Department of Energy missions, including the Stockpile
200-kilovolt switch and two 100-kilovolt capacitors. The bricks are
Stewardship Program of the National Nuclear Security Administration.
inside an annular enclosed metal cavity that looks like a giant Life
Savers candy, Stygar says.
Stygar is confident that Z 300 will quadruple pressures for conducting

material-physics experiments with plutonium, uranium and other
Z 300 will be driven by 90 LTD modules, each consisting of 33 LTD
critical elements; achieve thermonuclear ignition in an inertially confined
cavities (each cavity is 2 meters in diameter and .22 meters thick)
deuterium-tritium plasma; quadruple the energy and power radiated
stacked horizontally, like a Life Savers roll. Altogether, Z 300 will
by non-thermal X-ray sources for weapon-physics and weapon-effects
have 2,970 cavities, each producing a 100-nanosecond-long,
experiments; and quadruple the energy and power radiated by thermal
105-gigawatt power pulse.
X-ray sources for laboratory astrophysics, radiation opacity and

radiation transport experiments.
Each cavity converts, in a single step, the energy stored in its

capacitors to the 100-nanosecond pulse, Stygar says. Hence, Z 300
John Porter, senior manager of Sandias Z accelerator sciences group,
will not need any additional pulse compression hardware.
was the first to propose building a next-generation LTD accelerator

that fits inside the same building.
But it will need some work to upgrade LTD cavities from a 79-gigawatt
electrical pulse, the current standard, to the labs 105-gigawatt pulse
The High Current Electronics Institute (HCEI) at Tomsk, Russia, began
goal. To get there, technicians will replace existing switches with new,
work on LTD technology about 10 years ago. Sandia has developed the
more advanced ones now under development by researchers from
technology to its present state. Stygar, a Sandia researcher since 1982,
Kinetech Inc. and Sandia. Theyll also use upgraded capacitors from
says Russia, Israel, France, England, China and other countries already
technology company General Atomics. Voss Scientific also participates
use LTD technology to drive high energy density physics experiments.
in the project.
LTD technology dates back to 1920s, when Erwin Marx described his
Stygar says the plan is to first operate an LTD cavity at 105 gigawatts.
self-named generator. Thirty-six Marx generator-driven pulsed-power
Then the team of about 17 technicians and researchers will build an
modules create the 26-megampere, 80-terawatt pulse that powers Z.
LTD module with 33 cavities that generates a 3.5-terawatt electrical
A Marx generator creates a 1 microsecond-long power pulse. Z
power pulse. After we demonstrate successful operation of this
experiments, however, require a 100-nanosecond power pulse, so
module, we will be ready to build Z300.
Fitzpatrick
S TEWA R D S H I P S C I EN C E 13/ 14 TH E STony
S G F MA
G A ZI NE P5
FRONT LINES
Little Big Bang
Big Bang began our universe 13.8 billion years ago. By bashing
measurements, so theorists must instead conduct thought experiments.
together energized heavy gold or lead ions accelerated to
Those reconstruct QGP qualities by using particles formed after the
quipped with particle accelerator-colliders, scientists are

glimpsing conditions like those scant microseconds after the
near-light speed, they trigger so-called Little Bangs that help reveal
quarks and gluons recombine. Thats what makes the field exciting
states of matter that are even odder than theyd anticipated.
and at the same time difficult.
Los Alamos National Laboratory physicist Ivan Vitev is among the
Vitevs contributions began with a paper published in 2002, the year
theorists attempting to understand these tiny-bang states, known as
he received his doctoral degree from Columbia University. It laid the
quark-gluon plasmas, or QGPs. Thats because QGPs are by definition
theoretical foundation for jet tomography, which can be used once in a
not observable on the time scales at which detectors make experimental
blue moon, he says, whenever a comparatively rare heavy ion collision
measurements, Vitev says.
creates especially energetic quarks or gluons. One quark or gluon may

collide with another and bounce apart like billiard balls at azimuths
QGPs themselves refute normal rules of the strong interaction, a
roughly 180 degrees apart. After ricocheting, one of the resulting
fundamental force that keeps matters core components quarks and
particles continues on at a high speed and energy. The other rapidly
gluons bound in an unbreakable embrace. Scientists think the Big
loses both in a shower of fragments the jet while passing through
Bangs stupendous energy burst let quarks and gluons very briefly roam
and interacting with the detectors plasma medium.
free. But within a few microseconds, they cooled enough to rejoin as

the building blocks of protons, neutrons and other contemporary
Experimentalists can then study the measurable byproducts. For
fundamental particles.
example, if one of the particles is a rare Z boson or a photon, the data

can be tagged for comparison with the final byproduct of its counterpart.
Little Bang experiments artificially boost particle energy levels just
Researchers know those fragments are spaced by a predictable azimuth
enough to recreate those last moments when quarks and gluons were
and that one has interacted with the plasma medium, whereas the
still approximately free, Vitev says. These semi-liberated QGPs were
other hasnt. They can reliably use this information to recreate details
expected to be gaseous. But when the Relativistic Heavy Ion Collider
about the immeasurable QGP itself, such as its density and temperature.
(RHIC) at Brookhaven National Laboratory began producing them in
Vitev compares this method to positron emission tomography and
the summer of 2000, puzzled scientists instead found them acting
radiography because both those medical techniques create images by
like perfect liquids, flowing with practically no viscosity.
processing signals from particle behavior within a medium.
Such discoveries, also observed at CERN accelerators in Europe, have to
His theoretical work is part analytic and part computational, he
be interpreted by theory to extract the information, Vitev says. We
says, and his codes run on local computer clusters at Los Alamos,
have only a very short time about a millionth of a billionth of a second
where he started in 2004 as a J. Robert Oppenheimer Fellow and
when this plasma state lives and develops features we are looking
now works in the Theoretical Division.
for in experimental data. Thats too fleeting for accelerator detector
Monte Basgall
continued from page 4
Researchers can examine the pairs of nuclei that form as the nucleus
Although scission the last part of fission is incredibly important,
comes apart. Most break into a variety of combinations with different
its also the hardest to understand. Physicists would follow the
energies, so Younes and colleagues are interested in which fragments
process up to this point of no return but didnt have the tools to
form and how frequently. Understanding scission is so challenging,
examine the nucleus as it fragments. Younes and his team now use their
in part, because the breakup of a single nucleus into two doubles the
framework to examine scission and have gotten as far as calculating
complexity: two sets of properties now, plus the nuclei are interacting,
some properties of the resulting nuclear splinters.
introducing still another variable that can affect the system.
This visualizes jet quenching in a lead-lead collision in the Large Hadron Colliders ATLAS detector at a center of
mass energy of 2.76 TeV per nucleon-nucleon pair. Green and yellow bars represent particle tracks and energy
deposition into the detector subsystems. An energetic jet is clearly visible at 1 oclock. The gray cone shows
theres a jet (a large energy deposition in a narrow cone) in this direction. Its away-side partner at 7 oclock
is completely missing, having dissipated its energy into the plasma.
continued from page 4
ISOTOPE HOPES
Fields and her advisor, Juan Collar at the University of Chicago,

and Elliott are all collaborators on Majorana, an international
It will take some sensitive detectors to answer
experiment that will use germanium-76 to seek signs of neutrinoless
basic questions about the nature of matter
double-beta decay.
in the universe. Fellow Nicole Fields

project during her Los Alamos National
Laboratory practicum will help researchers
PARTICLE TRACKER
calibrate properties of a key material that

could do the job.
Joshua Renners practicum project at Livermore was the same as his

doctoral research at the University of California, Berkeley, only different.
Working with Steve Elliott and the Neutron Science and Technology
Groups weak interactions team, Fields examined germanium-76, an
In both, Renner worked on technology for time projection chambers, or TPCs,
isotope researchers hope will find evidence of neutrinoless double-beta
designed to detect evidence of neutrinoless double-beta decay. Its key to
decay. This rare particle interaction is key to understanding neutrinos
understanding neutrinos and to advance knowledge of the universe.
the chargeless, nearly massless byproducts of nuclear reactions and

advance knowledge of the universe.
TPCs track charged particles released when two larger particles collide
or, in some cases, when atoms of fissionable materials split. In essence,
But germanium-76, when above ground, may interact with naturally
the energetic particles scientists seek knock loose electrons from atoms of
occurring cosmic rays, creating radioactive contaminants that could
a gaseous material (the detector medium) in the TPC. The number of
interfere with experiments. The Los Alamos researchers wanted to test
freed electrons characterizes the particles energy.
other elements that produce similar radioactivity at much higher rates.

By counting gamma rays from those other materials, the researchers
At UC Berkeley and Lawrence Berkeley National Laboratory, Renner
could estimate how much cosmic ray exposure the germanium
worked under James Siegrist, now associate director of the Department
received and account for that in their measurements.
of Energy Office of Science for the High Energy Physics program. The
group collaborates with other institutions to develop a prototype
Fields exposed foils comprised of the other elements cadmium, zinc
detector using xenon as a detector medium thus the acronym
and niobium to neutron beams at the Los Alamos Neutron Science
NEXT, for Neutrino Experiment with a Xenon TPC.
Center to simulate cosmic ray exposure, but at higher levels. Then she
used a detector to count gamma rays and determine which and how
At Livermore, Renner worked with physicist Adam
many radioactive isotopes resulted. With the neutron flux that hit the
Bernstein on the negative ion TPC. It uses negative ion
foils and the measured cosmic ray neutron flux, Fields could predict
drift, in which freed electrons attach to gas particles,
which radioactive isotopes would be good indicators of neutron
forming negative ions. The ions drift through an electric
exposure from space.
Although the LLNL scientists are beginning to get a picture of what
particles. Scission is such an extreme example of the quantum
scission looks like, questions remain. For example, physicists continue to
many-body problem.
discuss the role of certain neutrons in the fission process. These scission
neutrons, in the neck of that splitting peanut, sometimes are emitted
Fission is the most computationally challenging problem in nuclear
as the nucleus breaks. We would like to be able to calculate what those
physics, Younes says, partly because it incorporates so many complex
neutrons are doing from a microscopic point of view, Younes says. On
dynamic phenomena. It produces a lot of different kinds of observables
the atomic scale, this fundamental science also could help researchers
and is incredibly rich in the type of phenomena that you can study.
understand a variety of scientific problems that come up with multiple
Sarah Webb
FRONT LINES
field to a region in which each electron can detach from its ion and
correlates with Rayleigh-Taylor instability growth. John also is learning
create a signal for counting.
a Caltech-developed multiscale computer model of strain-induced

phase transformations in materials like iron. With Caltech engineering
Renner learned computer simulation tools to emulate ion drift behavior.
professor Michael Ortizs group, shes creating simulations and
The simulations, operating under a set of assumptions about how
comparing them with the Omega experiments. Shell also use
detachment works, provided clues to maximizing the process in
the model to predict results from the gas gun experiments.
Livermores detector setup. Learning new computational skills was

useful, Renner says, but the experience of working on a new project
in a new setting proved unexpectedly valuable.
IONIC BRAKE-TAPPING
At Livermore, fellow Alex Zylstra helped set the course for aspects
HIGH-PRESSURE SITUATION
of his supervisors research and added a branch to his own path. The
Massachusetts Institute of Technology student worked with Gilbert
Her practicum at Livermore set Kristen John
Collins to design experiments probing transport properties in inertial
on the road to a high-pressure doctoral
confinement fusion implosions conducted at NIF. Current models are
thesis. John spent the summer working
untested because no one has proposed practical experiments in relevant
with Hye-Sook Park and Bruce Remington to
conditions that are able to run on todays facilities.
learn her way around laser-driven tests of

material strength under high pressures and
One set of Zylstras tests looks at electron-ion equilibration, the rate at
high strains. (See Laser Days of Summer,
which temperatures of the two implosion components even out. Varying
Stewardship Science 2012-13.)
temperatures between electrons and ions can substantially affect the

implosions observed behavior, Zylstra says, but experimental data is
The practicum became the foundation of her thesis and of a partnership
limited. Zylstra also designed trials to measure ion-stopping power
between the Livermore researchers and a group at her university, the
the way alpha particles lose energy in the implosion hot spot due to
California Institute of Technology, that included Johns advisor,
complex collision processes. The energy loss rate sets requirements on
Guruswami Ravichandran.
conditions for an ignition chain reaction, but experiments so far havent

measured ion-stopping power in strongly coupled or degenerate plasmas.
At Livermore, John designed experiments using laser-driven compression

to study solid-state material properties. She mastered two radiation
For both investigations, Zylstra simulated the radiation
hydrodynamics computer simulation codes, read papers and talked
hydrodynamics and made calculations to predict the
with colleagues. John also traveled four times to assist with experiments on
signal-to-noise ratio and quantify measurement accuracy.
Omega, the powerful laser at the University of Rochester, and helped

analyze the results. The experiments included a study of Rayleigh-Taylor
Zylstras practicum performance was outstanding, Collins
instability in tantalum.
says, and his projects helped define a roadmap to

benchmark transport properties and provided estimates
With that knowledge, John helped design experiments investigating
of uncertainty for these quantities.
irons properties under the high pressures achievable only at Omega

and the National Ignition Facility, known as NIF, Livermores giant laser
The practicum fit well with Zylstras MIT research under Richard
complex. The shots, carried out on Omega in summer 2012, indicate
Petrasso, whose group develops diagnostics for NIF and Rochesters
iron is stronger than simulations predicted, John says. Nonetheless,
Omega laser and explores the physics of fusion and general high
her thesis will focus on the tantalum experiments because theyre
energy density plasmas. The projects ion-stopping aspects, Zylstra
further along.
says, are now part of his doctoral thesis and evolved into a partnership
between the Livermore and MIT groups. The researchers carried out
John also is conducting experiments to recreate the Omega shots on
the first shots in the ion-stopping experiment earlier this year on
a small scale, using a Caltech gas gun to target ballistic gelatin and
Omega, and theyre planning for more.
tin. The goal is to observe how the materials flow and see if strength
Thomas R. ODonnell
BRIDGING SCIENCE,
POLICY AND THE PUBLIC
Certainly, working in Congress really drove
that point home. I learned that there is a critical
role for scientists to play in policy. There doesnt
have to be this barrier between the policymakers
and scientists.
C O N V E R S AT I O N
Laura Berzak Hopkins

Physicist, Lawrence Livermore

After that year, you could have stayed

in Washington and pursued a career in
science policy, but you chose to return
to the national lab system and opened my
to a research position at Lawrence
eyes to the career opportunities there. Also,
Livermore National Laboratory. How
my initial introduction to science policy came
did you make that decision?
through the fellowship. At our annual
National Laboratory
DOE NNSA SSGF Class of 2010
Its important to explain

why peoples tax dollars
should fund what scientists
are working on.
gatherings there always are opportunities

I am still excited about science and research,
for connections to policymakers in D.C.
so I wasnt certain I was ready to completely

step away from research. Livermore provides a
You recently co-founded a forum called
As a 2010-11 American Physical
lot of opportunities as far as career advancement
Why-Sci.com to connect nonscientists
Society Congressional Science
merging with science policy, so that was
with scientists and research. Why should
Fellow, you got an inside look at
definitely a big draw for me.
scientists communicate directly with
how science policy develops in

Washington. What did you take
the public?
What are you working on now?
away from your year in D.C.?
The reason its so important to build that

My graduate research was in magnetic fusion.
bridge is two-fold. In times of fiscal constraint
I think the general public has this idea
Now Im part of the research staff at the National
like we are in and will likely continue to be in,
that if you are a scientist you know all
Ignition Facility, so Im working in inertial fusion,
its important to explain why peoples tax
kinds of science. I was working in Congress
which to anyone outside the field is exactly
dollars should fund what scientists are working
when the Fukushima disaster unfolded. I
the same. But its completely different. Im
on. Second, its important for the public
was asked to write a memo explaining
studying different types of high energy density
to understand that from their new, quiet
the different features and factors involved
implosions driven by NIF, which is an enormous
refrigerator to their iPod, science goes into all
in the [Japanese] nuclear power plant
laser facility. The goal is to reach ignition,
of that. Its important for people to understand
and contrasting that to what the media
which is a self-sustaining burn of light fuel
that scientific research really does affect them
were reporting. I also would get questions
deuterium and tritium. Im in the design
and those investments can improve their lives.
because someone thought: This is
physics group, so I work on the type of target
science. You give it to the scientist. For
the laser hits and on shaping the laser pulse
One of the biggest take-home messages I
example, I did research on poppy growing
both in power and in time, which is an
learned in D.C. is that people are excited
in Afghanistan and how it affects the opium
important part of how the implosion performs.
about science. So many people I met in D.C.
trade. Thats certainly outside my sphere
who dont know about science were excited
of knowledge. But as scientists, we are
How did your time as an SSGF Fellow
to learn more. My office [former Sen. Kent
trained in research skills. Although we
inform your career choices?
Conrad, D-N.D.] asked me to give a lunchtime
apply them to our specific fields, I learned
mini-lecture on fusion and ongoing plasma
you also can apply those research skills
During my practicum I worked at Sandia National
physics experiments. It was exciting to see
to a variety of topics. There was a general
Laboratories, where I focused on developing
the interest, and I think part of it was the
comfort with getting research questions
advanced materials for plasma-facing
direct interaction with a scientist who was
that you dont know the answer to and
components in magnetic fusion reactors. That
willing to explain what they do. Thats the
figuring out how to answer them.
was an interesting and important introduction
model for Why-Sci.com.
COVER STORY
Lab initio
BY JACOB BERKOWITZ
Title image: Snapshot from a simulation of xenon in

which liquid atoms (red) are solidifying (green) at a
high temperature and pressure.
Jacob Berkowitz is a science writer and, most recently,
author of The Stardust Revolution: The New Story of
Our Origin in the Stars (Prometheus Books, 2012).
P 1 0 STEWARDSHIP SCIEN C E 1 3 / 1 4 T HE S S GF M AGAZ INE
Luke Shulenburger
Scientists at Sandia National Laboratories

are out to make first-principles chemical
models, hoping to reduce error and
illuminate experiments on materials
under extreme conditions.
hile in high school in Lawrence, Luke Shulenburger would bike or walk up the hill
to the University of Kansas, where professors mentored the precocious teen in
math, physics, chemistry and computer science.
By his senior year, this extracurricular education had led him to the National
Junior Science and Humanities Symposium and his first paper in Physics Letters A,
co-authored with his mentors and published when he was an undergraduate at the
Massachusetts Institute of Technology.
It also led him to a career-defining conundrum. While studying organic chemistry
and struggling to memorize reaction rules, he wondered why chemists didnt work
like physicists: mathematically, from fundamental first principles.
Why couldnt you just solve the equations behind everything? says Shulenburger,
now a staff scientist in the high energy density physics theory group at Sandia National
Laboratories in New Mexico. Ive been playing around with that ever since.
Today, Shulenburger has found his intellectual home. Hes part of a new generation
of young Stockpile Stewardship program researchers at National Nuclear Security
Administration laboratories who are driven to create models of matter based not
primarily on experimental data, but on first-principles physics equations ab initio,
literally from the beginning, models.
At the heart of this vision is Quantum Monte Carlo (QMC), a computational modeling
technique that grew from work at Los Alamos National Laboratory in the early
1950s. Sixty years later, QMC is finding its greatest expression in extreme parallel
computing applications on DOEs high-end supercomputers.
As a result, two decades since the last U.S. underground nuclear test, Shulenburger
and colleagues are taking stewardship science into a new era. They are harnessing
the combination of QMC techniques, dramatic new insights into materials at the
extreme and visions of ever more powerful computing to create a new race for
accuracy between experimentalists and theorists.
Experimental results will always be needed to ground our research, but our goal is
to provide a more complete picture, says Shulenburger, who presented his latest
QMC work at the American Physical Society meeting in March 2013.
BEYOND APPROXIMATIONS
Shulenburger wasnt the first to dream of theoretically predicting the physical and
chemical properties of matter from first principles. The pioneers of quantum theory
long shared that vision. The formulation of the Schrdinger equation describing the
quantum behavior of electrons held the promise of theoretically solving any chemical
interaction. In practice, however, the equation hits a computational Mount Everest.
Problems scale exponentially with the number of particles. Thus, even with enormous
computing power, exact solutions are obtainable only for molecules with just a
few electrons.
To vault this quantum multibody hurdle, computational scientists have developed
ways to approximate solutions to the Schrdinger equation. Each approximation
A visualization of a charge
density for solid argon,
calculated with quantum
Monte Carlo methods.
incorporating a mix of experimental

data and what physicists call physics
intuition makes the equation more
computationally tractable.
The problem is that every approximation
also distorts reality to some extent.
Thus, approximations are fertile
ground for improvement for the
Stockpile Stewardship Programs
Predictive Capability Framework,
which aims to significantly reduce
modeling uncertainties.
The common thread that links all
of my research is the elimination of
approximations to develop a more
precise ability to simulate materials
under extreme conditions,
Shulenburger says.
Since joining Sandia in 2010, Shulenburger
has taken a two-pronged approach to
reduce approximations in models of
elements across the periodic table
under extreme pressure.
First is adapting and applying QMCPACK,
a new QMC code optimized for use on
DOEs massively parallel leadership-class
computers. (See sidebar, New Code
Tested Against the Elements.)
The workhorse of quantum computational
approximation is density functional
theory, or DFT. The technique was
developed several decades ago and now
has thousands of users and applications
agile enough to run on smartphones.
But DFT falters in describing how matter
behaves under extreme conditions,
particularly for heavy atoms.
This is where QMCPACK enters the
picture. QMC uses a stochastic, random
step-sampling technique to solve wave
equations, an approach with a completely
different and potentially tinier class of
approximations than DFT.
NEW CODE TESTED AGAINST THE ELEMENTS
pair of young DOE scientists is confident that a
year, with Ceperley and colleagues, he co-wrote a
new first-principles quantum simulation code
paper on hydrogen and helium under extreme
will provide unprecedented predictive accuracy in
conditions for Reviews of Modern Physics.
modeling elements across the periodic table under

sun-like extremes of temperature and pressure.
Probably for the light elements, were there, says

Shulenburger, who recently used QMCPACK to
Miguel Morales
Their optimism is based on QMCPACK, for
reveal a possible new beryllium solid-solid phase
Quantum Monte Carlo Package. Quantum Monte
transition under high pressure. But as you get to
Carlo isnt a widespread method yet, says Miguel
the heavier elements, its much more difficult from
Morales, a staff scientist in the Condensed Matter
the computational point of view.
and Materials Division at Lawrence Livermore National
QMC is an excellent fit with stockpile

stewardship because it has the potential
to determine materials properties
with extremely small uncertainties,
Shulenburger says. This is critical to
verification and validation proving
models act as intended and reducing
uncertainty. With QMC you have the
opportunity to get the physics right
even where your intuition fails you.
QMC algorithms also are naturally
parallelizable on several levels, providing
the ideal models for petascale computers
that can do quadrillions of scientific
calculations a second and exascale
machines at least a thousand times
more powerful than those. If you give
me a bigger computer to run on and
fortunately the DOE has lots of big
computers I can make the statistical
approximation error as small as I want.
Although QMC provides one avenue
for reducing approximations, another
approach quantifies how much each of
those approximations potentially
skews simulations.
Many researchers working to improve
QMCs accuracy have focused on
reducing the fixed-node approximation,
known to limit ab initio calculations of
Laboratory. In terms of stockpile stewardship, the
In a 2010 Proceedings of the National Academy
challenge for us is to develop QMCPACK to the
of Sciences paper, Morales used QMC ab initio
point at which theres trust in its predictive capabilities.
simulations to confirm and pinpoint a liquid-liquid

transition in high-pressure hydrogen of interest to
QMCPACK was created under the leadership of
planetary scientists considering giant gas planets
the University of Illinois David Ceperley, a pioneer
like Jupiter.
in developing the quantum Monte Carlo family

of methods.
Morales and Shulenburger are working with Sandia

and Livermore colleagues to extend the QMCPACK
Ceperley, also a staff scientist at the universitys
benchmarking to other elements, including gold,
National Center for Supercomputing Applications,
silver and molybdenum. Applying QMCPACK includes
worked with fellow professor and physicist Richard
porting the code to other supercomputers, including
Martin to mentor a talented group of graduate
Cielo at Los Alamos and Sequoia, the IBM Blue
students. Many of those students now are Department
Gene/Q at Livermore.
of Energy staff scientists applying QMCPACK to the
most challenging stockpile stewardship problems.
The effort also has involved porting QMCPACK to

run on graphics processing units, or GPUs. These
Jeongnim Kim, a scientist in the Computational
massively parallel, energy-efficient chips developed
Chemistry and Materials Division at Oak Ridge
for video games are giving a low-cost, high-efficiency
National Laboratory, leads QMCPACKs
boost to high-performance computing. Notes
ongoing development.
Shulenburger, With GPUs you almost have to think

of your problem in a whole different way about
QMCPACK is completely designed with extreme
how to decouple everything into parallel tasks to an
parallelism in mind, Morales says. Test runs on
extent thats previously unheard of. The approach is
Oak Ridges petaflops-capable supercomputer
ideal for QMC, a naturally parallelizable technique.
showed the code could be scaled up to the entire

machine with little loss in efficiency. In a discipline
Titan, a world-leading computer at Oak Ridge, already
in which modeling a dozen individual electrons is
gets most of its processing power from GPUs. Kenneth
considered an admirable feat, QMCPACK has
Esler of Stone Ridge Technologies, another of
demonstrated its capable of modeling thousands
Ceperleys University of Illinois disciples, recently
of particles in a computationally cost-effective way.
ported QMCPACK to run on them.
Morales and Sandia National Laboratories Luke
Morales says the challenge QMCPACKs advocates
Shulenburger both of whom, along with Kim,
face is to build a series of success stories, convincing
worked with Ceperley on QMCPACK are testing
others of its accuracy and utility. To the extent that
the code in a benchmarking program to predictively
we can start using correct first-principle predictions
model elements under extreme conditions. Were
of materials at high density, we will start to identify
going to touch on elements across the periodic table
problems in stockpile stewardship models currently
and identify those areas where we do well and those
being used. There are still many hurdles to cross, but
where we need to work harder, Morales says. Last

I think its just a matter of time.
Shulenburgers come full circle in his

desire to get down to ab initio basics.
condensed matter and nuclear reactions. The approximation is a computational

compromise that addresses the fermion sign problem, one of the major unsolved
problems in modeling the physics of many-particle quantum systems.
In a system with two or more electrons, the wave function has regions with opposite
signs: one positive, the other negative. However, for efficiency, QMC typically
calculates only in an approximation of the positive space. This fixed-node approximation
is the most difficult to eliminate and is a fundamental uncertainty in QMC
calculations today.
Shulenburger and colleagues are pursuing a comprehensive solution to the sign
problem. Hes already made significant progress by showing that, in practice, it
might be less important than previously thought in solving important stockpile
stewardship problems. My work has found that it is rarely the determining factor
for high-accuracy simulations, Shulenburger says. The way we partition the
problem into tightly bound and chemically active pieces is far more important
than this more theoretically fundamental question.
QMC INSIGHTS TO MATTER AT THE EXTREME

Approximations notwithstanding, QMC already has proven its worth in revealing
a dramatically new map of matters terrain at extreme temperatures and pressures.
From first principles, says Lawrence Livermore National Laboratorys Miguel
Morales, weve identified a completely new set of states of matter that appear
when you compress materials, and many of these were completely unexpected.
Morales is a Livermore staff scientist and an alumnus of the DOE National Nuclear
Security Administration Stewardship Science Graduate Fellowship. Hes collaborating
with Shulenburger to systematically apply QMCPACK a code they both helped
develop as graduate students at the University of Illinois to predict the equations
of state for elements at high temperatures and pressures.
Theyve both witnessed the power of ab initio models to redefine our understanding
of material behaviors at the extreme conditions critical to stockpile stewardship
and fields such as planetary geophysics.
For example, previous models assumed that delocalized electrons ones at high
pressure, stripped from their nuclei form a uniform electron curtain ions interact
against. In practice thats not always what happens, Morales says. Instead, in atoms
from such elements as aluminum and sodium under extreme pressure, delocalized
electrons congregate in the voids of the ionic lattice, creating stable electride structures.
Similarly, Shulenburger says, scientists now are reassessing models of large atoms
that ignored inner electrons. One of the fascinating things about high-pressure
science is you can get to the point where

these previously chemically inert inner
electrons start to matter, because the
energy scales go up and up as you bring
the ions closer and closer together, and
factoring this in fundamentally changes
the properties of materials at these
extreme conditions.
Shulenburger was introduced to
real-world high-pressure materials
problems as a post-doctoral researcher
at the Carnegie Institutions Geophysical
Laboratory in Washington, D.C. There,
researchers study the behavior of minerals
squeezed at enormous pressures and
temperatures inside the Earth.
In his time at Sandia, Shulenburgers
come full circle in his desire to get down
to ab initio basics. Working closely with
Sandias engineers and experimentalists,
his QMC fine-tuning focuses on making
this first-principles technique useful in
the Stockpile Stewardship Programs
applied big picture.
When I was a grad student at Illinois, if I
could tell you about the phenomenon
of a solid under pressure, that it metalizes
and heres why, you probably wouldnt
have cared as much about exactly at
what temperature and pressure that
happened, he says. But at Sandia, where
an engineer may actually incorporate
those data into plans for a device, you
care a lot more about the details. So
Ive gotten a lot more focused in terms
of how to produce a high-precision
quantitative result rather than just
getting a qualitative sense of the
physics of a problem.
IN THEIR
ELEMENT
BY KARYN HEDE
Lawrence Livermore
National Laboratory
scientists are probing
properties of atoms on
the edge of the periodic
table. Their rapid
separation techniques
could have ramifications
for nuclear forensics.
For years
the periodic table

has existed in limbo, its otherwise orderly
stacks and rows of elements petering out at
the bottom with a series of elements that
seemed to signal chemists had exhausted
their ideas. Running across the lower right
row, the elements from No. 113 to No. 118
read as a series of Us. One might guess
these stood for unknown.
At least some of these orphans finally
now have names that acknowledge their
discovery. Element 114 is flerovium, after
the Flerov Laboratory of Nuclear Reactions in Dubna, Russia, where it was first
created. Likewise, No. 116 now is livermorium, after Lawrence Livermore National
Laboratory. The labs collaborated on the discoveries and still cooperate on pushing
the edge of the periodic table, seeking the outer limit of possible elements.
Perhaps no living scientist is more associated with element discovery than Livermores
Ken Moody, a radiochemist and member of Livermores super heavy element group.
Moody, who was involved in discovering elements 113 to 118, has spent years trying to
understand the central issue of how atomic nuclei balance the repulsion between
protons with the nuclear glue that binds them. Just how heavy can an element get,
he wonders, before clusters of positively charged protons prompt nuclear fission?
This lingering issue motivates nuclear chemists in the super heavy element group.
But the tools and technology required to address this fundamental question also
have found applications in nuclear forensics, actinide chemistry and other fields.
Once a new element is discovered, group
leader Dawn Shaughnessy says, the next
question is what are (its) chemical properties and
how does it relate to its neighboring elements in
the periodic table? Doing those experiments is
challenging because you are literally doing
chemistry on a single atom of something
that only lasts a short amount of time.
Their fleeting existence means we have scant
or, in some cases, no information about the
ions travel down an accelerator at
chemical properties of the heavy elements
a high velocity, about 30,000
occupying the last few blocks in period 7, the
kilometers per second, toward
last row on the periodic table. For example,
a rotating californium target.
we know that element 118 existed only by
measuring alpha particles released in its nearly immediate decay to livermorium
and then to flerovium. Its the same for nearly all the man-made elements: Scientists
only know theyve been there by counting radioactive emissions as they decay.
In this artists conception, calcium
Years ago, Moody described his work to his elementary school-aged daughter.
Her incredulous response You mean you dont actually know whether you have
anything until it goes away? encapsulates the difficulties of working with such
ephemeral species.
CHEMISTRY BY ANALOGY
Most super heavy elements can be studied only at the few places that have colliders
capable of firing ions calcium, generally at one of the actinide elements, such
as curium or californium, at speeds approaching 30,000 kilometers per second.
Experiments using these rarest of elements are both practically and financially
Karyn Hede is a freelance journalist whose work has appeared in Science,

Scientific American, New Scientist, Technology Review and elsewhere.
difficult, so the Livermore team wants

to probe the chemistry of analogous
elements in the same vertical group,
whose bonding and chemical behavior
should be similar. The idea is to perfect
analytical methods using elements that
can reliably be made in a standard ion
accelerator, then transfer those methods to
study the super heavy elements.
Given the challenge of understanding
the chemical behavior of an atom with
a half-life of less than a minute, the
Livermore researchers must develop swift
chemical methods and ways to automate
often-repetitive experiments. Dubnium,
for example, exists in several isotopes
that have half-lives from 35 seconds to
up to one day. The problem with the
more stable form of the element, which
is named for the Flerov Laboratorys
location, is that generally its possible to
generate only one atom of it per day.
We need a chemistry where the kinetics
are really fast, Shaughnessy says. It
may be that with a standard chemistry
on a stable element you can let your
experiment sit and equilibrate for a
long time. We dont have that luxury.
Livermore uses an automated device that
introduces a sample as a gas-borne aerosol
to a testing chamber, deposits it on a
porous glass frit, adds acids to convert
the sample into a liquid and rotates it
for subsequent chemical separation and
measurement. The device then moves
to a cleaning position and rotates back
to collect another sample. The device
allows the chemists to repeat an experiment
about once a minute for days or weeks,
Narek Gharibyan, a postdoctoral researcher,

works on chemical separations of heavy
elements at Lawrence Livermore National
like lead. It should behave like a noble gas, something inert that doesnt react.
And that would be a big deal in terms of how we understand the periodic table.
Laboratory. The lab is known for its skill at

separation methods, which are useful to
identify uranium sources.
gathering enough data to understand how

heavy elements such as Nos. 104, 105
and 106 adsorb or desorb from a surface.
Following the periodic table would
lead scientists to expect that dubnium
(element 105) shares properties with
tantalum (No. 73, just above dubnium
in period 6) and niobium (No. 41, two
rows up in period 5), Moody says.
The good news is that it does. But
the interesting thing is that you would
expect it to be more similar to tantalum
than niobium, just because it is closer
in atomic weight, but in some systems
we have found it is closer to niobium.
In some ways, the research pits periodic
table father Dmitri Mendeleev against
Albert Einstein. When a nucleus
becomes large enough, its positive
charge causes electrons orbiting it
to spin so fast that relativistic effects
make predicting its behavior difficult.
If you just put element 114 in the periodic
table it should sit under lead, Shaughnessy
says. But there are nuclear orbital
models that say it should not behave
The new element 118 travels through

the accelerator to a detector. Quickly
separating and observing the new atom
is key to understanding its properties.
The research groups goal is to understand how element 114, flerovium, behaves. To get
there, they are developing very fast chemistry using some of the lighter elements in
group 14, such as lead and tin. The researchers are studying ligands, binding agents
that can pull lead or tin out of a mixture. They also collaborate with Texas A&M
University and the University of Nevada, Las Vegas (UNLV) to study new materials
that will separate super heavy elements quickly and efficiently from interfering
background products. Several doctoral students have conducted their thesis research
on chemical extraction and on analyzing behavior down a specific group in the
periodic table.
FINDING AN ATOM IN A HAYSTACK

Livermore scientists mastered isotopic separation methods in an era of open-air
nuclear tests before 1962. For example, the labs Center for Accelerator Mass
Spectrometry can separate and count a handful of uranium-236 atoms from a
sample of several grams. Such exacting separations are essential when trying to
identify the source of uranium taken from one of dozens of sites where mined
ore is processed and enriched for energy production or weapons.
The challenge, Moody says, is taking decades of separations and analytical expertise and
applying it to the needs of modern nuclear forensics. In the 1960s, the research team had
time to carefully scrutinize a tests products. Today, the goal is to supply answers
that quickly locate the source of, for example, illegally obtained uranium. Perhaps
just as important, the researchers want to track the material sources should a terrorist
organization succeed in detonating a dirty bomb or other nuclear weapon. In a blast
scenario, the nuclear forensics group would analyze debris and reverse-engineer
what device was used and how it was built.
The problems you have doing the heavy element chemistry are often similar to the
problems you would have in a (nuclear) forensics type of scenario, Shaughnessy says.
You are looking for a very small amount of something in a large matrix of background
material. You want to separate it quickly because everything is radioactive, and you
want to get the answer as soon as possible. We are always looking for new methods
of very rapid separation techniques.
In recent years, Livermore also has cultivated expertise in developing chemical
signatures that let the scientists identify where and how a particular sample of
uranium was produced. Now theyre working on parsing how it gets to where its
seized. To that end, Livermore has teamed with UNLV researchers to rapidly
identify uranium samples. Graduate students and post-doctoral researchers
often split their time between the two locations.
Jonathan Plaue, one such doctoral student, recently discovered that different
uranium samples precipitated into unique and reproducible crystalline shapes
depending on their origin. This project, which formed an important part of his
dissertation, could help to rapidly identify interdicted samples from a specific
location or produced through a similar process.
If we had a real-world sample, we now believe that simply by looking at the shape
or shapes of the particles we may be able to infer the process or processes that were
used to produce those particles, says Ian Hutcheon, a physicist and leader of the
chemical & isotopic signatures group in Livermores Chemical Sciences Division.
Part of Hutcheons group specializes in the exacting work of measuring the
RARE EARTH
T
he rare appearance of a meteor streaking over Russia in 2013 shocked local

observers but offered scientists another chance to learn more about the origins of
the universe. For inside each slice of meteorite debris are some of the earliest building
blocks of solid matter once-molten droplets produced by high-temperature processes
at the birth of the solar system.
Few opportunities exist to study the remnants of such phenomena here on Earth, but
a recent discovery at Lawrence Livermore National Laboratory may have opened up a
new possibility.
Ian Hutcheon, a physicist who studies heterogeneous materials in the nanometer to
micrometer scales, was examining some of the glassy debris created during outdoor
nuclear testing in the 1950s and 60s. He realized that microscopic patterns in the
glassy spherules created moments after a powerful nuclear blast resemble those in
chondrules, the glassy spheres found in primitive meteorites.
It turns out that these fallout particles, even
though they are made of glass, are not
homogeneous, Hutcheon says. You find
abundances of uranium isotopes in

surprisingly complex, small samples.
(See sidebar, Rare Earth.)
Looking ahead, the research team aims
to avoid the chemical separation step
altogether. Instead, the researchers in
Hutcheons group are pointing lasers at
fallout samples to atomize them. An
ionizing laser fired at the cloud would
transform only the atoms of interest,
usually uranium or plutonium, into an
ionized state. Ideally, the uranium or
plutonium would absorb the photons,
with all other elements invisible, then
would be drawn into a mass spectrometer
for counting. The method also would be
applicable to all the actinide elements,
but to make it practical much more
information about the atomic energy
levels of these elements must be collected.
Toward that end, the group collaborates
with researchers at the Naval Post Graduate
School in Monterey, Calif., to study the
atomic energy levels of the heavy elements
in the actinide period the 15 elements
between Nos. 89 and 103. That includes
uranium to curium, the most interesting
ones for nuclear forensics.
large variations in both the elemental

composition and, even more intriguing,
in the isotopic composition. Hutcheons
research team found that within a single
marble-like spherule, pockets of uranium-235
Cross section of a 2 milimeter-diameter
(the isotope found in a nuclear device) and
glassy spherule produced during a nuclear
uranium-238 (the uranium form found in the
test, mounted in epoxy. On the left, an
environment) exist side-by-side and unmixed,
optical micrograph shows a large central
along with various blends of the two.
cavity surrounded by many smaller
We think that this new technique,

called resonance ionization mass
spectrometry, gives us the ability to do
analyses on the time scale of much less
than a day, Hutcheon says. The
required mass spectrometer will be
built at Livermore while the basic
research project is underway.
bubbles. On the right, a scanning electron

What this tells us is that these spherules
microscopic image shows variations in
were made in the aftermath of the detonation
chemical composition that reveal clues
by a process or processes that had to mix
to the rate of cooling and solidification.
materials coming from the device with
The light band at the perimeter is
material coming from the environment.
enriched in calcium and iron.
Hutcheons nearly 40 years of experience studying meteorite inclusions may provide

clues to the mixing processes that occur in the seconds after a nuclear blast. His
research could offer a new avenue for combining nuclear forensics with the physics
of early solar system formation.
Ultimately, Shaughnessy envisions a

mobile system that would make nuclear
forensics field-deployable.
We really should be thinking of
completely new technology, she says.
I could think of probably five projects
tomorrow that a student could go
launch on. That could make a huge
difference in nuclear forensics.
BY THOMAS R. ODONNELL
T he
BEAM COUNTERS
RESEARCHERS USING LOS ALAMOS
NATIONAL LABORATORYS TRIDENT
LASER HAVE GENERATED POTENT
NEUTRON PULSES, OPENING NEW
AVENUES FOR SCIENCE.
A Trident laser shot,

delivering as much as 200
quintillion watts of energy
per square centimeter to a
deuterium-carbon target.
HE INTERCOM ECHOES THROUGH THE TRIDENT LASER
FACILITY AT LOS ALAMOS NATIONAL LABORATORY. A technician

speaks. We are preparing for a system shot to the north target area. She warns staff
to avoid high-voltage hardware and the laser bay. Do not break any interlocks.
S TEWA R D S H I P S C I EN C E 13/ 14 TH E S S GF MA G A ZI NE P19
Researcher Markus Roth at work in the target

chamber at Los Alamos National Laboratorys
Trident laser, where scientists often join lab
technicians in preparing shots.
The sheer number of energetic neutrons,

delivered in incredibly short bursts,
makes the Trident beams suitable for
multiple uses, from deciphering the
fundamentals of radiation damage to
identifying illicit nuclear materials. The
technology also may advance neutron
research as institutions without the space
and money for linear accelerators embrace
compact neutron-generating lasers.
Scientists Juan Fernndez and Markus Roth listen from a nearby office. Fernndez
leads Los Alamos experimental plasma physics group. Roth is a laser plasma
physicist from Germanys Technical University of Darmstadt. Shots are always
a little bit like a rocket launch, Roth says. But instead of sending off satellites,
Trident is firing oodles of high-energy neutrons.
Its February, and Roth is taking a break between shot setups on his second
Trident visit in under a year. In spring and summer 2012, he was a Rosen Scholar,
serving a research fellowship at LANSCE, the Los Alamos Neutron Science Center.
LANSCE includes the Lujan Center, where a kilometer-long accelerator generates
neutron beams for investigating materials, protein structures, nanomaterials and
other subjects.
Some of what the Lujan Center does in a kilometer, Trident now does in a few
millimeters, thanks to a collaboration involving Roth, Fernndez and other
researchers from Germany and from Los Alamos and Sandia National Laboratories.
The 2012 experiments produced the largest neutron beams a short-pulse laser has
ever made: An object placed a centimeter from the source would get a burst of
neutrons at a density of 4 quintillion 1018 per square centimeter per second.
Those neutrons also move fast, with energies as high as 150 megaelectron volts
(MeV, or a million electron volts). Conventional accelerator technology like that
at the Lujan Center delivers many more neutrons but over a long period. That
makes the two techniques complementary, Fernndez says.
Thomas R. ODonnell, senior science editor, has written extensively about

research at the DOE national laboratories. He is a former science reporter
at The Des Moines Register.
Thats probably the most exciting

aspect, says Frank Merrill, a neutron
scientist and team leader for the
advanced imaging group in Los
Alamos Physics Division. Its this
novel way of generating neutrons
that may open applications nobody
has thought about because (neutron
beams) were so expensive to generate
and build.
Tridents unusual properties and some
physics wizardry make it possible.
LASER JOCKS
The voice on the intercom indicates the
power level of capacitors that soon will
discharge in Tridents high-intensity
beam. Twenty-five percent charge.
Fernndez and Roth, Merrill says, are
laser jocks: physicists who know how
to use short-pulse lasers to do all kinds
of fascinating things. Although the
two collaborators are unsure about the
nickname No self-respecting laser
scientist would call us laser jocks,
Fernndez jokes they agree lasers are
key to their research. Juan and I are
more the users, Roth says. We really
are the experimental side.
Merrills specialty is detectors to count

neutrons and measure their energies. He
and his colleagues develop sensitive
diagnostics for the National Ignition
Facility, or NIF, the giant laser built at
to implode tiny hydrogen-filled capsules
and, if successful, trigger nuclear fusion.
NIF is in demand and shots are difficult
and expensive, so routinely using the
laser to test diagnostics isnt feasible.
Merrill and his collaborators need a
NIF stand-in: someplace that readily
generates copious neutrons in a
short pulse.
Trident, a neodymium glass laser, can
deliver 200 trillion watts of energy in
pulses as short as half a picosecond,
a trillionth of a second. Roth says its
reputation as one of the worlds best
short-pulse laser systems drew him to
Los Alamos. Although hes a plasma
physicist, I had neutrons always on
my mind and worked on previous
attempts to produce them with lasers.
Older systems, however, werent
powerful enough to yield significant
numbers or energies.
ON TARGET
Fifty percent charge.
Compared to larger laser facilities, like NIF and the University of Rochesters
Omega, research at Trident is more hands-on, Fernndez and Roth say. Los Alamos
technicians are involved, but the scientists themselves often work together to set
up targets and instruments, getting their hands dirty, Fernndez says. Graduate
students work alongside them to make as many shots as possible in a day. Roth
adds, To sum it up, we are having a party here. He laughs. Its really a great
team, but of course we are working hard.
For the neutron beam experiment, Trident targets a super-thin plastic foil. Few
big lasers can use such foils because of prepulse a weak but significant burst of
light that heats or destroys the target beforethe main pulse can hit it. Trident is
known for its high contrast, meaning the prepulse is negligible. You can shoot
targets that are very thin, Fernndez says, so you can move the whole foil at
once, as opposed to a fraction. That helps to accelerate the resulting plasma
ions to unprecedented energies.
The foils other key property is its composition: carbon and deuterium, a hydrogen
isotope that pairs a neutron with each atoms lone proton. The researchers focus
Tridents beam tightly and fire it in just trillionths of a second, hitting the foil with
200 quintillion watts of energy per square centimeter, equivalent to focusing all the
suns light into a spot the size of a pencils tip. The target is reduced to a plasma of
electrons and deuterons deuterium nuclei, comprised of one neutron and one proton.
The physics legerdemain that occurs next is vital to creating a powerful neutron
beam without a giant linear accelerator. Most plasmas are opaque to lasers; they
reflect the beam like a mirror. But under Tridents high intensity, plasma generated
from the foil becomes relativistically transparent, Roth and Fernndez say. It
Merrill, of course, also had neutrons on

his mind. Roth, after arriving at the lab
last year, gave a seminar on his plans.
Merrill caught him later in a hallway.
The Los Alamos detector researcher
needed a source for bright neutron
pulses. The German visitor wanted to
show lasers could provide them. A team
assembled to find a solution.
Experiments at the Trident laser hit a thin,

carbon-deuterium foil with an intense laser pulse,
driving deuterium nuclei into a beryllium rod. The
nuclei displace beryllium neutrons and also break
apart, generating an intense neutron beam.
Like a cue ball hitting a clump of billiard balls,

the deuterons send beryllium neutrons flying.
starts when electromagnetic waves from the laser light push electrons into the
target. The number of electrons available steadily decreases as theyre pushed
to the back of the foil.
At the same time, the laser intensity ramps up, Roth says. The electrons have
to oscillate in that electromagnetic wave. Because the intensity is so high, the
electrons are accelerated to the speed of light, stop, accelerated to the speed
of light, stop, at every cycle of the laser pulse. That means most of the time
electrons are accelerated to near light speed.
Heres where Einstein steps in. Under relativity, electrons become heavy as they
accelerate. With laser intensity increasing, theyre no longer able to follow the
beam because to stop a very heavy electron takes a longer time than to stop a light
electron, Roth says. In quadrillionths of a second, the electrons can no longer
follow the electromagnetic waves, the foil becomes transparent and the beam
passes. Suddenly, the laser breaks through that foil and catches up with the
electrons that are already pulling on the ions on the other side. The laser couples
efficiently to all electrons in the volume, not just those on the plasma surface.
The researchers call this effect breakout afterburner the laser breaks through
the foil and transfers energy through the electrons to the deuterons, accelerating
them in a burst. The linked proton and neutron slam into a shielded beryllium
rod placed just 5 millimeters beyond the foil.
Beryllium atoms have a large cross section, meaning their neutrons have a high
probability of interacting with incoming protons and neutrons. Like a cue ball
hitting a clump of billiard balls, the deuterons send beryllium neutrons flying.
Meanwhile, some deuterons break apart, generating additional neutrons, Merrill
says. You get some added oomph. What we found is you get higher-energy
neutrons from that piece of the process.
The neutron beam could be even bigger, Fernndez says, if the foils were pure or
nearly pure frozen deuterium an idea Roth plans to try later this year.
For Merrill and his detector-developing colleagues, the tough part was finding the
neutrons amid the noise X-ray and electromagnetic radiation byproducts. They
sifted them with a time-gated system, essentially a high-speed shutter that opens
after X-rays pass but before neutrons arrive. We could find the sweet spot,
admitting the neutrons of interest while in essence, everything else was quiet.
P 2 2 STEWA RD SH IP SCIENC E 1 2 / 1 3 T HE S S GF M AGAZ INE
If anything, the laser researchers

did their jobs too well, Merrill says,
producing neutrons at energies greater
than he and his colleagues need for
NIF neutron detectors. (See sidebar,
Capturing Neutrons.)
ON THE PHYSICS EDGE

Seventy-five percent charge.
Before these experiments, Trident had
never accelerated deuterium ions. This
whole relativistic regime is really the
edge of the known physics, Roth says.
But the researchers had some guidance:
Theorists at Los Alamos Computational
Physics Division, including Brian Albright,
Chengkun Huang, Lin Yin and Huichun
Wu, predicted optimum target thicknesses
for a given laser intensity. That helped the
experimentalists generate neutrons on
the first shot, not counting two others
done to check alignment. I knew Trident
A Trident shot as seen through a target

chamber port. The laser is known for its
high contrast, meaning it has little or no
prepulse a short, weak burst of light
before the main laser pulse.
CAPTURING NEUTRONS
was a great laser, but I never would have

dreamed that wed get results on the
third shot on the first day, Roth says.
here already are neutron detectors at NIF, the National Ignition Facility,
Frank Merrill says, but researchers need better ones.
In a sense, the instruments are like digital cameras. A camera with more pixels captures a finer
Although far smaller than a linear

accelerator, Trident still isnt portable
because its a multipurpose research facility.
A system designed specifically to generate
neutrons could fit on a truck, making
the technology available for a range of
research and practical uses, including
stockpile stewardship experiments.
image. A detector with better resolution provides a more accurate picture of neutron generation
and distribution in NIF shots.

NIF implosions are little tiny things, involving capsules of about 100 microns in diameter, says
Merrill, team leader for the Advanced Imaging Group in Los Alamos National Laboratorys Physics
Division. You dont want to just see theres a neutron source 100 microns in diameter. You want to
see some of the details inside. Top resolution now is about 10 microns and researchers are
constantly investigating ways to improve it. It would be wonderful if we got to 1 micron, but thats
a fairly significant technical challenge, he adds.
One use is flash radiography to assemble

detailed movies of mass evolution over
tiny time increments. With a neutron
source firing 60-nanosecond pulses,
Merrill says, researchers could string
together freeze-frames of fast, dynamic
events like how metal deforms under
an explosive force. Because materials
absorb neutrons at different energies,
beams also could peer inside materials
in ways X-rays cant. Neutron radiography
tells researchers not only how much of
a material is present the mass but
also what kind of material it is perhaps
aluminum in one part and steel in another.
In a similar way, the high-intensity,
high-energy beams Trident produces
are suited for active interrogation
scanning containers to spot hidden
nuclear materials, perhaps at ports and
border crossings. Detectors could track
particles and radiation emitted when a
neutron beam passes through a container,
providing investigators signatures of
materials inside, says research team
member Andrea Favalli, a scientist in
Los Alamos Nuclear Engineering and
Nonproliferation Division. Hes studying
the Trident beam for active interrogation
applications. Other such systems have
been tested, says Favalli, a native Italian,
including one he helped develop at the
Joint Research Centre of the European
With bright neutron sources like the one Merrill and other researchers developed at Los Alamos
Trident laser, detector scientists will have greater access to testing. But in some ways, Trident is too
good. NIF typically produces neutrons with energies of around 14 megaelectron volts (MeV). The
laser-driven neutrons at Los Alamos are up to 150 MeV. Its nice to have the higher energies,
Merrill says, but we were interested in the sweet spot, kind of zero to 30 MeV.
Never fear: The scientists use a high-tech gating system essentially a precise shutter to filter
out the speediest neutrons. Since they move faster, they arrive at the detectors first. Neutrons the
scientists seek come a hair later only after theshutter opens. That gated system is how we
were able to only look at the energy range we were interested in, Merrill adds.
Commission. Those, however, often relied on multiple measurements or measurements

over long periods. The laser-driven beam could generate neutron signatures with a
single rapid burst. There are many, many possible applications and more are
coming, Favalli says.
The current round of shots, in fact, is studying active interrogation. The team found
that passing the beam through a depleted uranium sample clearly delayed many of
the neutrons. Delayed neutrons is a signature of fission, indicating the presence of a
nuclear material.
***
One hundred percent.
Shot 23-73 is complete. All areas are clear.
With that and many other shots, research on the Trident neutron beam continues.
Many are part of Favallis active interrogation project, but scientists also will study
optimizing the pulse to produce neutrons with a specific range of peak energies,
Merrill says. The researchers also will address fluctuations in the number of
neutrons each pulse generates.
SAMPLINGS
Bottling the Sun

BY EVAN DAVIS
Evan Davis
A metallic feminine voice rings out through the control room:
melting the walls, the plasma temperature must drop from hundreds
Three. Two. One. Zero. Entering pulse. Dozens of scientists and engineers
of millions of degrees in the core to a few thousand at the reactor
hold their breath and fix their eyes on the large computer display at the
wall, creating one of the largest thermal gradients in the universe.
front of the room. A warm, guttural hum fills the air, the ground
softly vibrates, and a flash of light appears on monitors throughout
Unfortunately, small-scale turbulence allows the plasma to leak through
the room.
the tokamaks magnetic fields. Indeed, Nobel laureate Richard Feynman

once described confining plasma within a tokamak as trying to hold Jell-O
In fractions of a second, millions of watts of power heat dilute gas to
with rubber bands: its possible, but its taxing and youll probably lose at
200 million degrees Fahrenheit, 10 times the temperature of the suns
least part of the Jell-O. A dozen or so scientists work on C-Mod with the
core. At this temperature, the gas atoms are stripped of their electrons
express purpose of understanding and controlling this turbulence.
and their positively charged nuclei whiz by at 1 million miles per

hour. Some of these nuclei smash into each other with just the right
Researchers at C-Mod and several other tokamaks over the past two
orientation and speed to fuse, forming an altogether different nucleus
decades have identified several desirable operating modes that suppress
and releasing an enormous amount of energy.
these detrimental turbulent fluctuations. In particular, weve discovered

that the potential fusion gain in tokamaks is strongly controlled by
The pulse ends almost as soon as it began. The gas cools, the glow fades
parameters in the last inch or so of the plasmas edge.
from the monitors, and scientists scramble to analyze the data. Ten
minutes until next shot, the voice states, reminding the researchers
My colleagues and I are working to develop and test a first-principles
they must work quickly so theyre ready to coax every last bit of
computer model of this edge turbulence so that we can predict and
performance out of their machine in the next experiment.
optimize a devices performance before its even built. Developing such a

model requires a strong coupling between experiment, computation,
Its a typical day of operation at the Massachusetts Institute of
and theory. That means youll find me scrambling to set-up C-Mods
Technologys Alcator C-Mod reactor, located down a humble side street
phase contrast interferometer before the days experiments begin
in urban Cambridge, Mass. C-Mod is a compact nuclear fusion reactor
and fervently analyzing the measured turbulent density fluctuations
designed to study the scientific and engineering challenges that must
between shots. In the evenings, I run edge turbulence simulations on
be overcome to make this technology a viable energy source.
the worlds most powerful supercomputers, aiming to validate the

code by comparing it with my experimental measurements. Its a
Fusion is the energy of the sun and stars. Many scientists and engineers,
long, arduous process, but this crucial element of physics must be
including my MIT colleagues and me, want to bottle the sun for power
understood if were to advance to a viable reactor.
generation on Earth. When fully developed, fusion will provide

continuous power from abundant, virtually inexhaustible fuels, such
Fusion science has progressed exponentially since its inception, and
as deuterium, a hydrogen isotope harvested from seawater. Fusion
we now stand poised to make a viable reactor for the first time. An
power plants will not directly produce any greenhouse gases. They
international collaboration is constructing ITER, the first device
also would produce no long-lived nuclear waste, and there is no risk
expected to reach and exceed fusion breakeven the point at which
of a meltdown or nuclear materials spreading for use in weapons.
energy put into the reaction equals the energy it produces.
Tokamaks like C-Mod are the leading candidates for successful fusion
C-Mod is the only tokamak that operates at the same densities and
reactor designs. These doughnut-shaped vacuum vessels use powerful
heat fluxes as those expected in ITER, so its thrilling to be here
magnetic fields (2 to 3 Tesla, about the strength used in typical magnetic
and extremely important that our research continue.
resonance imaging (MRI) medical devices) to suspend a plasma in space,

preventing the hot core from touching any material walls. To prevent
The author is a third-year fellow at the Massachusetts Institute of

Technology and this his winning entry in the 2013 SSGF Essay Slam.
DOE NNSA SSGF FELLOWS
CLASS OF 2013
MATTHEW BUCKNER
School: University of North Carolina,
Chapel Hill
Discipline: Nuclear Astrophysics
Advisors: Thomas Clegg and Christian Iliadis
Practicum: Lawrence Livermore
National Laboratory
Contact: emcuebe@gmail.com
THOMAS SALLER
School: University of Michigan
Discipline: Nuclear Engineering
Advisor: Thomas Downar
Practicum: Sandia National
Laboratories, California
Contact: tgsaller@umich.edu
MAREENA ROBINSON
School: Massachusetts Institute
of Technology
Discipline: Nuclear Science and Engineering
Advisor: Richard Lanza
National Laboratory
Contact: mrobin@mit.edu
THIRD YEAR
HONG SIO
of Technology
Discipline: Plasma Physics
Advisor: Richard Petrasso
Contact: hsio@mit.edu
NICOLE FIELDS
School: University of Chicago
Discipline: Astroparticle Physics
Advisor: Juan Collar
Practicum: Los Alamos National Laboratory
Contact: fields@uchicago.edu
ADAM CAHILL
School: Cornell University
Advisor: David Hammer
Practicum: Los Alamos National Laboratory
Contact: adc87@cornell.edu
KRISTEN JOHN
School: California Institute of Technology
Discipline: Aerospace Engineering
Advisor: Guruswami Ravichandran
National Laboratory
Contact: kjohn@caltech.edu
JOHN GIBBS
School: Northwestern University
Discipline: Materials Science
Advisor: Peter Voorhees
National Laboratory
Contact: jgibbs917@gmail.com
JOSHUA RENNER
School: University of California, Berkeley
Discipline: Nuclear/Particle Physics
Advisor: James Siegrist
National Laboratory
Contact: josh.renner@berkeley.edu
GEOFFREY MAIN
School: Stanford University
Discipline:Computational Mathematics
Advisor: Charbel Farhat
National Laboratory
Contact: alexmain@stanford.edu
ALEX ZYLSTRA
of Technology
Discipline: Physics
Advisor: Richard Petrasso
National Laboratory
Contact: azylstra@psfc.mit.edu
WALTER PETTUS
School: University of Wisconsin, Madison
Discipline: Experimental Nuclear and
Particle Physics
Advisor: Karsten Heeger
National Laboratory
Contact: pettus@wisc.edu
FOURTH YEAR
EVAN DAVIS
of Technology
Discipline: Plasma Physics and Fusion
Advisor: Miklos Porkolab
National Laboratory
Contact: emd@mit.edu
MICHAEL HAY
School: Princeton University
Advisor: Nathaniel Fisch
National Laboratory
Contact: hay@princeton.edu
STEPHANIE LYONS
School:University of Notre Dame
Discipline: Nuclear Physics
Advisor: Michael Wiescher
National Laboratory
Contact: slyons3@nd.edu
ELIZABETH MILLER
School: Northwestern University
Discipline: Materials Science and Engineering
Advisor: Scott Barnett
Practicum: Sandia National Laboratories,
New Mexico and California
Contact: elizabethmiller2015@
u.northwestern.edu
DIRECTORY
JENNIFER SHUSTERMAN
Discipline: Nuclear Chemistry
Advisor: Heino Nitsche
National Laboratory
Contact: Jennifer.Shusterman@berkeley.edu
CHRISTOPHER YOUNG
School: Stanford University
Discipline: Plasma Physics/Thermosciences
Advisor: Mark Cappelli
National Laboratory
Contact: cvyoung@stanford.edu
SECOND YEAR
SAMANTHA LAWRENCE
School: Purdue University
Discipline: Materials Science and Engineering
Advisor: David Bahr
Practicum: Sandia National
Laboratories, California
Contact: slawrence.wsu@gmail.com
J. SCOTT MORELAND
School: Duke University
Discipline: Heavy-ion Nuclear Theory
Advisor: Steffen Bass
Contact: morelandjs@gmail.com
SSGF PROGRAM
Coordinator: Lucille Kilmer Contact: kilmer@krellinst.org
SABRINA STRAUSS
School: University of Notre Dame
Discipline: Physics
Advisor: Ani Aprahamian
Contact: systrauss@att.net
FIRST YEAR
BENJAMIN GALLOWAY
School: University of Colorado-Boulder
Discipline: Atomic, Molecular,
Optical Physics
Advisor: Margaret Murnane
Contact: Benjamin.r.galloway@colorado.edu
FABIO IUNES SANCHES
Discipline: Physics
Advisor: Undetermined
Contact: Fabioh.sanches@yahoo.com
IO KLEISER
School: California Institute of Technology
Discipline: Astrophysics
Advisor: Christian Ott
Contact: ikleiser@caltech.edu
JUAN MANFREDI
School: Michigan State University
Advisor: Betty Tsang
Contact: manfredi@frib.msu.edu
SARAH PALAICH
School: University of California, Los Angeles
Discipline: Geochemistry
Advisor: Abby Kavner
Contact: palaich@ucla.edu
FORREST DOSS
Discipline: Experimental Astrophysics
Fellowship Years: 2006-2010
Current Status: Staff Scientist, Los Alamos
National Laboratory
PAUL ELLISON
Discipline: Physical Chemistry
Current Status: Postdoctoral Fellow,
University of Wisconsin-Madison
ANNA ERICKSON (NIKIFOROVA)
of Technology
Discipline: Nuclear Engineering
Current Status: Assistant Professor,
Georgia Institute of Technology
MATTHEW GOMEZ
Discipline: Plasma Physics and Fusion
Current Status: Staff Scientist, Sandia
National Laboratories, New Mexico
RICHARD KRAUS
School: Harvard University
Discipline: Planetary Science
Current status: Finishing degree,
Harvard University
JORDAN MCDONNELL
School: University of Tennessee, Knoxville
Discipline: Theoretical Physics
Current status: Postdoctoral Fellow,
MIGUEL MORALES
School: University of Illinois at
Urbana-Champaign
Discipline: Theoretical Condensed
Matter Physics
Current Status: Staff Scientist, Lawrence
Livermore National Laboratory
ALUMNI
PATRICK OMALLEY
School: Rutgers University
Discipline: Experimental Nuclear Physics
Colorado School of Mines
LAURA BERZAK HOPKINS

School: Princeton University
Current Status: Physicist, Lawrence
Livermore National Laboratory
LUKE ROBERTS
School: University of California, Santa Cruz
Discipline: High Energy Astrophysics
Current Status: Finishing degree,
University of California, Santa Cruz
KRYSTLE CATALLI
of Technology
Discipline: Geophysics
Current Status: Failure Analysis
Engineer, Apple
ANGELO SIGNORACCI
School: Michigan State University
Commissariat lnergie atomique
(CEA), France
PAUL DAVIS
Discipline: Applied Physics
Advisor: Roger Falcone
Practicum: Sandia National Laboratories,
New Mexico
Contact: pfdavis@berkeley.edu
DYLAN SPAULDING
Discipline: Geophysics/Planetary Science
Harvard University
TAW INSPIRING
The game of marbles reached its

zenith in the 1950s and 60s, giving
birth to the term taw, for a glass
sphere of exceptional quality. This taw
2 millimeters across, much smaller
than a standard marble was made
in the same era but is the hardest of
all to come by: Its the byproduct of
outdoor nuclear weapons testing.
Lawrence Livermore National
Laboratory scientists discovered
that spherules like this one make
good earthly stand-ins for primitive
meteorites, which yield information
about the chemical makeup of the
early solar system. They also provide
clues to the mixing processes right
after a nuclear blast, offering a
potentially powerful new tool in
nuclear forensics. Further details
appear on page 18.
The Krell Institute | 1609 Golden Aspen Drive, Suite 101

Ames, IA 50010 | (515) 956-3696 | www.krellinst.org/ssgf

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STEWARDSHIP

Department of Energy National Nuclear Security Administration

$36,000 yearly stipend

Payment of full tuition and required fees

$1,000 yearly academic allowance

Yearly program review

12-week research practicum

Renewable up to four years

FOR MORE INFORMATION

Krell Institute | 1609 Golden Aspen Drive, Suite 101

National Nuclear Security Administration

LETTER FROM NNSA

Investing in the Future

With assistance from Mark Visosky

THE BEAM COUNTERS

STEWARDSHIP SCIENCE GRADUATE FELLOWSHIP

P 2 ST E WA RD SH IP SCIENCE 1 3 / 1 4 T HE S S GF M AGAZ INE

Deciphering the details of atom splitting.

24 BOTTLING THE SUN

Sandia plans to amp up the Z machine in the same space.

of turbulence that has an outsized say

6 LITTLE BIG BANG

Probing the properties of the quark-gluon plasma.

SCIENCE, POLICY AND THE PUBLIC

25 DOE NNSA SSGF FELLOWS

Former fellow Laura Berzak Hopkins on providing science expertise to

Where to find current fellows

Congress, fusions two varieties and her Why-Sci communications project.

SSGF STEERING COMMITTEE

lthough it releases vast amounts of energy, the process

Members of DOE National Nuclear Security Administration

of splitting atomic nuclei is still difficult to understand

Undaunted, Lawrence Livermore National Laboratory researchers are

Matthew Buckners practicum at Lawrence

looking at fissions microscopic detail with the hope of improving

Livermore National Laboratory was a bit like a

nuclear waste management and recycling and increasing nuclear power

high-tech physicists shop class. His plans for an

production. Describing fission in detail also can help answer basic

improved gas ionization chamber detector went

science questions, such as how heavy elements formed in the universe.

from computer modeling to fabrication

Physicists started delving into fission theoretically 75 years ago by

Buckner worked with Scott Tumey at Livermores Center for Accelerator

neutrons within the nucleus, they considered it as a liquid drop,

Mass Spectrometry. Accelerator mass spectrometry, or AMS, speeds ions

to high energies, separating isotopes from surrounding material before

Younes says. During

mass analysis. AMS is used in several fields, including detecting signatures

fission, the drop would

of nuclear fuel reprocessing an important nonproliferation function.

stretch into an oblong

The device Buckner made uses AMS to measure transition metal

the scission point,

activation products. He simulated a previous design on a computer

the narrow neck in

the peanut would

anodes to adequately collect electrons. After some research, he used

break to form two